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Time delays in two-photon ionization

  • Jing Su
  • , Hongcheng Ni
  • , Agnieszka Jaroń-Becker
  • , Andreas Becker
  • University of Colorado Boulder

科研成果: 期刊稿件文章同行评审

摘要

We present results of ab initio numerical simulations of time delays in two-photon ionization of the helium atom using the attosecond streaking technique. The temporal shifts in the streaking traces consist of two contributions, namely, a time delay acquired during the absorption of the two photons from the extreme-ultraviolet field and a time delay accumulated by the photoelectron after photoabsorption. In the case of a nonresonant transition, the absorption of the two photons is found to occur without time delay. In contrast, for a resonant transition a substantial absorption time delay is found, which scales linearly with the duration of the ionizing pulse. The latter can be related to the phase acquired during the transition of the electron from the initial ground state to the continuum and the influence of the streaking field on the resonant structure of the atom.

源语言英语
期刊论文编号263002
期刊Physical Review Letters
113
26
DOI
出版状态已出版 - 24 12月 2014
已对外发布

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