Organically doped palladium: A highly efficient catalyst for electroreduction of CO2 to methanol

Heng Pan Yang; Sen Qin; Huan Wang; Jia Xing Lu

doi:10.1039/c5gc01504a

Organically doped palladium: A highly efficient catalyst for electroreduction of CO₂ to methanol

Heng Pan Yang
, Sen Qin
, Huan Wang^*
, Jia Xing Lu

^*此作品的通讯作者

化学与分子工程学院

East China Normal University

科研成果: 期刊稿件 › 文章 › 同行评审

67 引用（Scopus）

摘要

A [PYD]@Pd composite was prepared by the entrapment of a pyridine derivative within metallic palladium. Metallic Pd acts as a heterogeneous support and a pyridine ring served as an active site for electroreduction of CO₂, and no additional catalyst was needed in the electrolyte. 35% Faradaic efficiency of methanol was obtained at only -0.6 V vs. SCE. Moreover, [PYD]@Pd has remarkable stability and reusability.

源语言	英语
页（从-至）	5144-5148
页数	5
期刊	Green Chemistry
卷	17
期	12
DOI	https://doi.org/10.1039/c5gc01504a
出版状态	已出版 - 31 7月 2015

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abstract = "A [PYD]@Pd composite was prepared by the entrapment of a pyridine derivative within metallic palladium. Metallic Pd acts as a heterogeneous support and a pyridine ring served as an active site for electroreduction of CO2, and no additional catalyst was needed in the electrolyte. 35\% Faradaic efficiency of methanol was obtained at only -0.6 V vs. SCE. Moreover, [PYD]@Pd has remarkable stability and reusability.",

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AU - Yang, Heng Pan

AU - Qin, Sen

AU - Wang, Huan

AU - Lu, Jia Xing

PY - 2015/7/31

Y1 - 2015/7/31

N2 - A [PYD]@Pd composite was prepared by the entrapment of a pyridine derivative within metallic palladium. Metallic Pd acts as a heterogeneous support and a pyridine ring served as an active site for electroreduction of CO2, and no additional catalyst was needed in the electrolyte. 35% Faradaic efficiency of methanol was obtained at only -0.6 V vs. SCE. Moreover, [PYD]@Pd has remarkable stability and reusability.

AB - A [PYD]@Pd composite was prepared by the entrapment of a pyridine derivative within metallic palladium. Metallic Pd acts as a heterogeneous support and a pyridine ring served as an active site for electroreduction of CO2, and no additional catalyst was needed in the electrolyte. 35% Faradaic efficiency of methanol was obtained at only -0.6 V vs. SCE. Moreover, [PYD]@Pd has remarkable stability and reusability.

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DO - 10.1039/c5gc01504a

M3 - 文章

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JO - Green Chemistry

JF - Green Chemistry

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Organically doped palladium: A highly efficient catalyst for electroreduction of CO2 to methanol

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Organically doped palladium: A highly efficient catalyst for electroreduction of CO₂ to methanol