Optical refrigeration of the Yb³⁺-doped YAG crystal close to the thermoelectric cooling limit

The Yb3+:YAG crystal has been one of the most widely used active media in the solid-state lasers of high power, mainly thanks to its excellent thermal, mechanical, and optical properties. Thermal effect due to heat deposition in the active medium, however, greatly deteriorates the beam quality of the laser output and sets a limit on its maximum power available. Although the cooling proposal of anti-Stokes fluorescence can help realize the heat-free high-power lasers with good beam quality, so-called radiation-balanced lasers, there is no substantial advancement in the optical cooling of Yb3+:YAG crystals since its latest experimental report with a temperature drop of about 9 K. Here we demonstrate experimentally a remarkable temperature drop of about 80 K in a 3% Yb3+-doped YAG single crystal pumped by a fiber laser at 1030 nm. Further analysis predicts that the cooling limit of the titled crystal can reach as low as 180 K from the room temperature. Our work therefore reveals a key pathway to facilitate the optical refrigeration of the Yb3+:YAG crystal down to the thermoelectric cooling limit, thus offering a unique entry point to practical radiation-balanced lasers.