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Molecular rotational effects in free-space N+2 lasers induced by strong-field ionization

  • Jinping Yao
  • , Bin Zeng
  • , Wei Chu
  • , Haisu Zhang
  • , Jielei Ni
  • , Hongqiang Xie
  • , Ziting Li
  • , Chenrui Jing
  • , Guihua Li
  • , Huailaing Xu
  • , Ya Cheng*
  • *此作品的通讯作者
  • CAS - Shanghai Institute of Optics and Fine Mechanics
  • State Key Laboratory on Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University

科研成果: 书/报告/会议事项章节章节同行评审

摘要

Free-space N2+ lasers induced by strong-field ionization have shown a great potential for the standoff diagnostics of quantum rotational wave packets in air molecules and for the fingerprint identification of chemical species, thanks to their capability of remotely generating intense, narrow-bandwidth, coherent emissions. It has been observed that the laser signals are strongly influenced by the dynamics of the rotational wave packets in the N2+ ions produced by photoionization in the intense laser fields. This chapter gives an overview of the experimental results of the effects of molecular rotations in the free-space N2+ lasers. We will begin with the description of the ultrafast dynamics of coherent rotational wave packets using the N2+ laser as an optical probe. We will follow with a discussion of the coherent coupling of the rotational quantum states in a strong laser field, manipulation of the polarization of N2+ laser emission, and the observation of impulsive rotational Raman scattering induced by the N2+ laser. Finally, a summary and perspective will be given.

源语言英语
主期刊名Springer Series in Optical Sciences
出版商Springer Verlag
75-88
页数14
DOI
出版状态已出版 - 2018

出版系列

姓名Springer Series in Optical Sciences
208
ISSN(印刷版)0342-4111
ISSN(电子版)1556-1534

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