Intense multiphoton upconversion of Yb3+-Tm3+ doped β-NaYF4 individual nanocrystals by saturation excitation

Jiajia Zhou; Gengxu Chen; Yingbin Zhu; Lili Huo; Wei Mao; Danna Zou; Xinwen Sun; E. Wu; Heping Zeng; Junjie Zhang; Long Zhang; Jianrong Qiu; Shiqing Xu

doi:10.1039/c4tc02363c

Intense multiphoton upconversion of Yb³⁺-Tm³⁺ doped β-NaYF₄ individual nanocrystals by saturation excitation

Jiajia Zhou
, Gengxu Chen
, Yingbin Zhu
, Lili Huo
, Wei Mao
, Danna Zou
, Xinwen Sun
, E. Wu
, Heping Zeng
, Junjie Zhang
, Long Zhang
, Jianrong Qiu
, Shiqing Xu^*

^*此作品的通讯作者

China Jiliang University
East China Normal University
Singapore University of Technology and Design
CAS - Shanghai Institute of Optics and Fine Mechanics
Zhejiang University

科研成果: 期刊稿件 › 文章 › 同行评审

59 引用（Scopus）

摘要

Saturation excitation of individual nanocrystals represents a powerful strategy to explore unique optical characteristics of luminescent activators. Here we report the intense multiphoton upconversion of β-NaYF₄: Yb³⁺-Tm³⁺ individual nanocrystals benefiting from the perfect ladder-type electron configuration of Tm³⁺ under saturation illumination excitation. This leads to a luminescence switching between the emissions from 2-photon upconversion and 4-photon upconversion, which exhibits significantly enhanced luminescence intensity by up to a factor of 70. Such intense multiphoton upconversion may have potential application in super-resolution imaging.

源语言	英语
页（从-至）	364-369
页数	6
期刊	Journal of Materials Chemistry C
卷	3
期	2
DOI	https://doi.org/10.1039/c4tc02363c
出版状态	已出版 - 14 1月 2015
已对外发布	是

访问文件

10.1039/c4tc02363c

其它文件与链接

链接到 Scopus 的出版物

引用此

@article{29155206209941fdbc8b6227fa798c02,

title = "Intense multiphoton upconversion of Yb3+-Tm3+ doped β-NaYF4 individual nanocrystals by saturation excitation",

abstract = "Saturation excitation of individual nanocrystals represents a powerful strategy to explore unique optical characteristics of luminescent activators. Here we report the intense multiphoton upconversion of β-NaYF4: Yb3+-Tm3+ individual nanocrystals benefiting from the perfect ladder-type electron configuration of Tm3+ under saturation illumination excitation. This leads to a luminescence switching between the emissions from 2-photon upconversion and 4-photon upconversion, which exhibits significantly enhanced luminescence intensity by up to a factor of 70. Such intense multiphoton upconversion may have potential application in super-resolution imaging.",

author = "Jiajia Zhou and Gengxu Chen and Yingbin Zhu and Lili Huo and Wei Mao and Danna Zou and Xinwen Sun and E. Wu and Heping Zeng and Junjie Zhang and Long Zhang and Jianrong Qiu and Shiqing Xu",

note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry 2015.",

year = "2015",

month = jan,

day = "14",

doi = "10.1039/c4tc02363c",

language = "英语",

volume = "3",

pages = "364--369",

journal = "Journal of Materials Chemistry C",

issn = "2050-7526",

publisher = "Royal Society of Chemistry",

number = "2",

}

TY - JOUR

T1 - Intense multiphoton upconversion of Yb3+-Tm3+ doped β-NaYF4 individual nanocrystals by saturation excitation

AU - Zhou, Jiajia

AU - Chen, Gengxu

AU - Zhu, Yingbin

AU - Huo, Lili

AU - Mao, Wei

AU - Zou, Danna

AU - Sun, Xinwen

AU - Wu, E.

AU - Zeng, Heping

AU - Zhang, Junjie

AU - Zhang, Long

AU - Qiu, Jianrong

AU - Xu, Shiqing

PY - 2015/1/14

Y1 - 2015/1/14

N2 - Saturation excitation of individual nanocrystals represents a powerful strategy to explore unique optical characteristics of luminescent activators. Here we report the intense multiphoton upconversion of β-NaYF4: Yb3+-Tm3+ individual nanocrystals benefiting from the perfect ladder-type electron configuration of Tm3+ under saturation illumination excitation. This leads to a luminescence switching between the emissions from 2-photon upconversion and 4-photon upconversion, which exhibits significantly enhanced luminescence intensity by up to a factor of 70. Such intense multiphoton upconversion may have potential application in super-resolution imaging.

AB - Saturation excitation of individual nanocrystals represents a powerful strategy to explore unique optical characteristics of luminescent activators. Here we report the intense multiphoton upconversion of β-NaYF4: Yb3+-Tm3+ individual nanocrystals benefiting from the perfect ladder-type electron configuration of Tm3+ under saturation illumination excitation. This leads to a luminescence switching between the emissions from 2-photon upconversion and 4-photon upconversion, which exhibits significantly enhanced luminescence intensity by up to a factor of 70. Such intense multiphoton upconversion may have potential application in super-resolution imaging.

UR - https://www.scopus.com/pages/publications/84917710808

U2 - 10.1039/c4tc02363c

DO - 10.1039/c4tc02363c

M3 - 文章

AN - SCOPUS:84917710808

SN - 2050-7526

VL - 3

SP - 364

EP - 369

JO - Journal of Materials Chemistry C

JF - Journal of Materials Chemistry C

IS - 2

ER -

Intense multiphoton upconversion of Yb3+-Tm3+ doped β-NaYF4 individual nanocrystals by saturation excitation

摘要

访问文件

其它文件与链接

指纹

引用此

Intense multiphoton upconversion of Yb³⁺-Tm³⁺ doped β-NaYF₄ individual nanocrystals by saturation excitation