Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

H. Sann; T. Havermeier; C. Müller; H. K. Kim; F. Trinter; M. Waitz; J. Voigtsberger; F. Sturm; T. Bauer; R. Wallauer; D. Schneider; M. Weller; C. Goihl; J. Tross; K. Cole; J. Wu; M. S. Schöffler; H. Schmidt-Böcking; T. Jahnke; M. Simon; R. Dörner

doi:10.1103/PhysRevLett.117.243002

Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

H. Sann
, T. Havermeier
, C. Müller
, H. K. Kim
, F. Trinter
, M. Waitz
, J. Voigtsberger
, F. Sturm
, T. Bauer
, R. Wallauer
, D. Schneider
, M. Weller
, C. Goihl
, J. Tross
, K. Cole
, J. Wu
, M. S. Schöffler
, H. Schmidt-Böcking
, T. Jahnke
, M. Simon

R. Dörner

Goethe University Frankfurt
University of Marburg
Sorbonne Université

科研成果: 期刊稿件 › 文章 › 同行评审

30 引用（Scopus）

摘要

We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.

源语言	英语
文章编号	243002
期刊	Physical Review Letters
卷	117
期	24
DOI	https://doi.org/10.1103/PhysRevLett.117.243002
出版状态	已出版 - 6 12月 2016
已对外发布	是

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Sann, H., Havermeier, T., Müller, C., Kim, H. K., Trinter, F., Waitz, M., Voigtsberger, J., Sturm, F., Bauer, T., Wallauer, R., Schneider, D., Weller, M., Goihl, C., Tross, J., Cole, K., Wu, J., Schöffler, M. S., Schmidt-Böcking, H., Jahnke, T., ... Dörner, R. (2016). Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation. Physical Review Letters, 117(24), 文章 243002. https://doi.org/10.1103/PhysRevLett.117.243002

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title = "Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation",

abstract = "We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.",

author = "H. Sann and T. Havermeier and C. M{\"u}ller and Kim, \{H. K.\} and F. Trinter and M. Waitz and J. Voigtsberger and F. Sturm and T. Bauer and R. Wallauer and D. Schneider and M. Weller and C. Goihl and J. Tross and K. Cole and J. Wu and Sch{\"o}ffler, \{M. S.\} and H. Schmidt-B{\"o}cking and T. Jahnke and M. Simon and R. D{\"o}rner",

note = "Publisher Copyright: {\textcopyright} 2016 American Physical Society.",

year = "2016",

month = dec,

day = "6",

doi = "10.1103/PhysRevLett.117.243002",

language = "英语",

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Sann, H, Havermeier, T, Müller, C, Kim, HK, Trinter, F, Waitz, M, Voigtsberger, J, Sturm, F, Bauer, T, Wallauer, R, Schneider, D, Weller, M, Goihl, C, Tross, J, Cole, K, Wu, J, Schöffler, MS, Schmidt-Böcking, H, Jahnke, T, Simon, M & Dörner, R 2016, 'Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation', Physical Review Letters, 卷 117, 号码 24, 243002. https://doi.org/10.1103/PhysRevLett.117.243002

TY - JOUR

T1 - Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

AU - Sann, H.

AU - Havermeier, T.

AU - Müller, C.

AU - Kim, H. K.

AU - Trinter, F.

AU - Waitz, M.

AU - Voigtsberger, J.

AU - Sturm, F.

AU - Bauer, T.

AU - Wallauer, R.

AU - Schneider, D.

AU - Weller, M.

AU - Goihl, C.

AU - Tross, J.

AU - Cole, K.

AU - Wu, J.

AU - Schöffler, M. S.

AU - Schmidt-Böcking, H.

AU - Jahnke, T.

AU - Simon, M.

AU - Dörner, R.

PY - 2016/12/6

Y1 - 2016/12/6

N2 - We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.

AB - We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.

UR - https://www.scopus.com/pages/publications/85003443820

U2 - 10.1103/PhysRevLett.117.243002

DO - 10.1103/PhysRevLett.117.243002

M3 - 文章

AN - SCOPUS:85003443820

SN - 0031-9007

VL - 117

JO - Physical Review Letters

JF - Physical Review Letters

IS - 24

M1 - 243002

ER -

Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

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