Dual-interface engineering strategy for optimizing carrier dynamics in perovskite-silicon tandem solar cells

Quanxing Ma; Yifan Chen; Zhou Liu; Xinxin Lian; Ming Luo; Shaobing Xiong; Jike Ding; Wenhuan Gao; Xueling Zhang; Yi Mo; Qinye Bao; Shengfan Wu; Yifeng Chen; Zhiqiang Feng; Xiaoliang Mo; Cong Chen; Junhao Chu; Hong Zhang

doi:10.1007/s40843-025-3630-2

Dual-interface engineering strategy for optimizing carrier dynamics in perovskite-silicon tandem solar cells

投稿的翻译标题: 钙钛矿-硅串联太阳能电池载流子动力学优化的双界面工程策略

Quanxing Ma
, Yifan Chen
, Zhou Liu
, Xinxin Lian
, Ming Luo
, Shaobing Xiong
, Jike Ding
, Wenhuan Gao
, Xueling Zhang
, Yi Mo
, Qinye Bao
, Shengfan Wu
, Yifeng Chen
, Zhiqiang Feng
, Xiaoliang Mo^*
, Cong Chen^*
, Junhao Chu
, Hong Zhang^*

^*此作品的通讯作者

物理与电子科学学院

Fudan University
Hebei University of Technology
Ltd.
Lingnan University

科研成果: 期刊稿件 › 文章 › 同行评审

摘要

This study demonstrates a dual-interface engineering approach for performance enhancement in perovskite-silicon tandem solar cells. By applying ethylenediamine dihydroiodide (EDAI₂) to simultaneously modify both top and bottom interfaces of wide-bandgap perovskite layers, we achieve synergistic defect suppression and charge transport optimization. Time-resolved photoluminescence characterization reveals extended carrier lifetimes and improved spatial homogeneity in dual-modified perovskite films. The optimized single-junction wide-bandgap (>1.66 eV) perovskite solar cells attain a champion efficiency of 22.75% with enhanced operational stability. Implemented in perovskite-silicon tandem configuration, the devices achieve over 31% power conversion efficiency, validating the effectiveness of organic ligand-mediated dual-interface engineering in regulating carrier dynamics and advancing perovskite-based tandem photovoltaics. (Figure presented.).

投稿的翻译标题	钙钛矿-硅串联太阳能电池载流子动力学优化的双界面工程策略
源语言	英语
页（从-至）	812-821
页数	10
期刊	Science China Materials
卷	69
期	2
DOI	https://doi.org/10.1007/s40843-025-3630-2
出版状态	已出版 - 2月 2026

访问文件

10.1007/s40843-025-3630-2

其它文件与链接

链接到 Scopus 的出版物

引用此

Ma, Q., Chen, Y., Liu, Z., Lian, X., Luo, M., Xiong, S., Ding, J., Gao, W., Zhang, X., Mo, Y., Bao, Q., Wu, S., Chen, Y., Feng, Z., Mo, X., Chen, C., Chu, J., & Zhang, H. (2026). Dual-interface engineering strategy for optimizing carrier dynamics in perovskite-silicon tandem solar cells. Science China Materials, 69(2), 812-821. https://doi.org/10.1007/s40843-025-3630-2

@article{0def2779675643a0b5a7a7b1ef44fbeb,

title = "Dual-interface engineering strategy for optimizing carrier dynamics in perovskite-silicon tandem solar cells",

abstract = "This study demonstrates a dual-interface engineering approach for performance enhancement in perovskite-silicon tandem solar cells. By applying ethylenediamine dihydroiodide (EDAI2) to simultaneously modify both top and bottom interfaces of wide-bandgap perovskite layers, we achieve synergistic defect suppression and charge transport optimization. Time-resolved photoluminescence characterization reveals extended carrier lifetimes and improved spatial homogeneity in dual-modified perovskite films. The optimized single-junction wide-bandgap (>1.66 eV) perovskite solar cells attain a champion efficiency of 22.75\% with enhanced operational stability. Implemented in perovskite-silicon tandem configuration, the devices achieve over 31\% power conversion efficiency, validating the effectiveness of organic ligand-mediated dual-interface engineering in regulating carrier dynamics and advancing perovskite-based tandem photovoltaics. (Figure presented.).",

keywords = "interface engineering, perovskite-silicon tandem solar cell, wide bandgap perovskite",

author = "Quanxing Ma and Yifan Chen and Zhou Liu and Xinxin Lian and Ming Luo and Shaobing Xiong and Jike Ding and Wenhuan Gao and Xueling Zhang and Yi Mo and Qinye Bao and Shengfan Wu and Yifeng Chen and Zhiqiang Feng and Xiaoliang Mo and Cong Chen and Junhao Chu and Hong Zhang",

note = "Publisher Copyright: {\textcopyright} Science China Press 2026.",

year = "2026",

month = feb,

doi = "10.1007/s40843-025-3630-2",

language = "英语",

volume = "69",

pages = "812--821",

journal = "Science China Materials",

issn = "2095-8226",

publisher = "Science China Press ",

number = "2",

}

Ma, Q, Chen, Y, Liu, Z, Lian, X, Luo, M, Xiong, S, Ding, J, Gao, W, Zhang, X, Mo, Y, Bao, Q, Wu, S, Chen, Y, Feng, Z, Mo, X, Chen, C, Chu, J & Zhang, H 2026, 'Dual-interface engineering strategy for optimizing carrier dynamics in perovskite-silicon tandem solar cells', Science China Materials, 卷 69, 号码 2, 页码 812-821. https://doi.org/10.1007/s40843-025-3630-2

TY - JOUR

T1 - Dual-interface engineering strategy for optimizing carrier dynamics in perovskite-silicon tandem solar cells

AU - Ma, Quanxing

AU - Chen, Yifan

AU - Liu, Zhou

AU - Lian, Xinxin

AU - Luo, Ming

AU - Xiong, Shaobing

AU - Ding, Jike

AU - Gao, Wenhuan

AU - Zhang, Xueling

AU - Mo, Yi

AU - Bao, Qinye

AU - Wu, Shengfan

AU - Chen, Yifeng

AU - Feng, Zhiqiang

AU - Mo, Xiaoliang

AU - Chen, Cong

AU - Chu, Junhao

AU - Zhang, Hong

PY - 2026/2

Y1 - 2026/2

N2 - This study demonstrates a dual-interface engineering approach for performance enhancement in perovskite-silicon tandem solar cells. By applying ethylenediamine dihydroiodide (EDAI2) to simultaneously modify both top and bottom interfaces of wide-bandgap perovskite layers, we achieve synergistic defect suppression and charge transport optimization. Time-resolved photoluminescence characterization reveals extended carrier lifetimes and improved spatial homogeneity in dual-modified perovskite films. The optimized single-junction wide-bandgap (>1.66 eV) perovskite solar cells attain a champion efficiency of 22.75% with enhanced operational stability. Implemented in perovskite-silicon tandem configuration, the devices achieve over 31% power conversion efficiency, validating the effectiveness of organic ligand-mediated dual-interface engineering in regulating carrier dynamics and advancing perovskite-based tandem photovoltaics. (Figure presented.).

AB - This study demonstrates a dual-interface engineering approach for performance enhancement in perovskite-silicon tandem solar cells. By applying ethylenediamine dihydroiodide (EDAI2) to simultaneously modify both top and bottom interfaces of wide-bandgap perovskite layers, we achieve synergistic defect suppression and charge transport optimization. Time-resolved photoluminescence characterization reveals extended carrier lifetimes and improved spatial homogeneity in dual-modified perovskite films. The optimized single-junction wide-bandgap (>1.66 eV) perovskite solar cells attain a champion efficiency of 22.75% with enhanced operational stability. Implemented in perovskite-silicon tandem configuration, the devices achieve over 31% power conversion efficiency, validating the effectiveness of organic ligand-mediated dual-interface engineering in regulating carrier dynamics and advancing perovskite-based tandem photovoltaics. (Figure presented.).

KW - interface engineering

KW - perovskite-silicon tandem solar cell

KW - wide bandgap perovskite

UR - https://www.scopus.com/pages/publications/105027236672

U2 - 10.1007/s40843-025-3630-2

DO - 10.1007/s40843-025-3630-2

M3 - 文章

AN - SCOPUS:105027236672

SN - 2095-8226

VL - 69

SP - 812

EP - 821

JO - Science China Materials

JF - Science China Materials

IS - 2

ER -

Dual-interface engineering strategy for optimizing carrier dynamics in perovskite-silicon tandem solar cells

摘要

访问文件

其它文件与链接

指纹

引用此