Down-conversion phosphors as noble-metal-free co-catalyst in ZnO for efficient visible light photocatalysis

Haipeng Chu; Xinjuan Liu; Jiaqing Liu; Wenyan Lei; Jinliang Li; Tianyang Wu; Ping Li; Huili Li; Likun Pan

doi:10.1016/j.apsusc.2016.07.031

Down-conversion phosphors as noble-metal-free co-catalyst in ZnO for efficient visible light photocatalysis

Haipeng Chu
, Xinjuan Liu^*
, Jiaqing Liu
, Wenyan Lei
, Jinliang Li
, Tianyang Wu
, Ping Li
, Huili Li
, Likun Pan

^*此作品的通讯作者

China Jiliang University
East China Normal University
Shanghai Nanotechnology Promotion Center

科研成果: 期刊稿件 › 文章 › 同行评审

16 引用（Scopus）

摘要

Exploring novel visible light responsive photocatalysts is one of greatly significant issues from the viewpoint of using solar energy. Here we report the yellow-orange emitting α-Si ₃ N ₄ -doped Lu ₃ Al ₅ O ₁₂ :Ce ³⁺ (Lu ₃ Al _5-x Si _x O _12-x N _x :Ce ³⁺ ) phosphors as a noble-metal-free co-catalyst for enhanced visible light photocatalytic activity of ZnO. The results show that ZnO-Lu ₃ Al _5-x Si _x O _12-x N _x :Ce ³⁺ hybrid photocatalysts using a fast microwave-assisted approach exhibits a 91% methylene blue (MB) degradation under visible light irradiation at 240 min, which evidence the synergistic effect of ZnO and Lu ₃ Al _5-x Si _x O _12-x N _x :Ce ³⁺ that suppress the rate of charge recombination and increase the self-sensitized degradation of MB. ZnO-down conversion phosphors can be envisaged as potential candidate in environmental engineering and solar energy applications.

源语言	英语
页（从-至）	468-475
页数	8
期刊	Applied Surface Science
卷	391
DOI	https://doi.org/10.1016/j.apsusc.2016.07.031
出版状态	已出版 - 1 1月 2017
已对外发布	是

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title = "Down-conversion phosphors as noble-metal-free co-catalyst in ZnO for efficient visible light photocatalysis",

abstract = " Exploring novel visible light responsive photocatalysts is one of greatly significant issues from the viewpoint of using solar energy. Here we report the yellow-orange emitting α-Si 3 N 4 -doped Lu 3 Al 5 O 12 :Ce 3+ (Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ ) phosphors as a noble-metal-free co-catalyst for enhanced visible light photocatalytic activity of ZnO. The results show that ZnO-Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ hybrid photocatalysts using a fast microwave-assisted approach exhibits a 91\% methylene blue (MB) degradation under visible light irradiation at 240 min, which evidence the synergistic effect of ZnO and Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ that suppress the rate of charge recombination and increase the self-sensitized degradation of MB. ZnO-down conversion phosphors can be envisaged as potential candidate in environmental engineering and solar energy applications.",

keywords = "Down conversion phosphors, Microwave-assisted approach, Photocatalysts, ZnO",

author = "Haipeng Chu and Xinjuan Liu and Jiaqing Liu and Wenyan Lei and Jinliang Li and Tianyang Wu and Ping Li and Huili Li and Likun Pan",

note = "Publisher Copyright: {\textcopyright} 2016 Elsevier B.V.",

year = "2017",

month = jan,

day = "1",

doi = "10.1016/j.apsusc.2016.07.031",

language = "英语",

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TY - JOUR

T1 - Down-conversion phosphors as noble-metal-free co-catalyst in ZnO for efficient visible light photocatalysis

AU - Chu, Haipeng

AU - Liu, Xinjuan

AU - Liu, Jiaqing

AU - Lei, Wenyan

AU - Li, Jinliang

AU - Wu, Tianyang

AU - Li, Ping

AU - Li, Huili

AU - Pan, Likun

PY - 2017/1/1

Y1 - 2017/1/1

N2 - Exploring novel visible light responsive photocatalysts is one of greatly significant issues from the viewpoint of using solar energy. Here we report the yellow-orange emitting α-Si 3 N 4 -doped Lu 3 Al 5 O 12 :Ce 3+ (Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ ) phosphors as a noble-metal-free co-catalyst for enhanced visible light photocatalytic activity of ZnO. The results show that ZnO-Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ hybrid photocatalysts using a fast microwave-assisted approach exhibits a 91% methylene blue (MB) degradation under visible light irradiation at 240 min, which evidence the synergistic effect of ZnO and Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ that suppress the rate of charge recombination and increase the self-sensitized degradation of MB. ZnO-down conversion phosphors can be envisaged as potential candidate in environmental engineering and solar energy applications.

AB - Exploring novel visible light responsive photocatalysts is one of greatly significant issues from the viewpoint of using solar energy. Here we report the yellow-orange emitting α-Si 3 N 4 -doped Lu 3 Al 5 O 12 :Ce 3+ (Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ ) phosphors as a noble-metal-free co-catalyst for enhanced visible light photocatalytic activity of ZnO. The results show that ZnO-Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ hybrid photocatalysts using a fast microwave-assisted approach exhibits a 91% methylene blue (MB) degradation under visible light irradiation at 240 min, which evidence the synergistic effect of ZnO and Lu 3 Al 5-x Si x O 12-x N x :Ce 3+ that suppress the rate of charge recombination and increase the self-sensitized degradation of MB. ZnO-down conversion phosphors can be envisaged as potential candidate in environmental engineering and solar energy applications.

KW - Down conversion phosphors

KW - Microwave-assisted approach

KW - Photocatalysts

KW - ZnO

UR - https://www.scopus.com/pages/publications/84994048948

U2 - 10.1016/j.apsusc.2016.07.031

DO - 10.1016/j.apsusc.2016.07.031

M3 - 文章

AN - SCOPUS:84994048948

SN - 0169-4332

VL - 391

SP - 468

EP - 475

JO - Applied Surface Science

JF - Applied Surface Science

ER -

Down-conversion phosphors as noble-metal-free co-catalyst in ZnO for efficient visible light photocatalysis

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