Continuous-Wave mid-Infrared to Visible Frequency Upconversion with a Molecular Optomechanical Nanocavity

W. Chen; P. Roelli; H. Hu; S. Verlekar; S. P. Amirtharaj; A. I. Barreda; T. J. Kippenberg; M. Kovylina; E. Verhagen; A. Martínez; C. Galland

Continuous-Wave mid-Infrared to Visible Frequency Upconversion with a Molecular Optomechanical Nanocavity

W. Chen
, P. Roelli
, H. Hu
, S. Verlekar
, S. P. Amirtharaj
, A. I. Barreda
, T. J. Kippenberg
, M. Kovylina
, E. Verhagen
, A. Martínez
, C. Galland^*

^*此作品的通讯作者

Swiss Federal Institute of Technology Lausanne
Wuhan Institute of Technology
Friedrich Schiller University Jena
Polytechnic University of Valencia
AMOLF

科研成果: 期刊稿件 › 会议文章 › 同行评审

摘要

We develop a plasmonic nanoparticle-in-groove nanocavity coupled with a few hundred molecules, demonstrating optomechanical transduction of sub-microwatt continuous wave signals from the mid-infrared (32 THz) onto the visible domain at ambient conditions. The dual resonant nanocavity offers an estimated 13 orders of magnitude enhancement in upconversion efficiency per molecule. Our results establish molecular cavity optomechanics as a new paradigm for coherent frequency conversion free of phase matching constraints.

源语言	英语
页（从-至）	703-704
页数	2
期刊	International Conference on Metamaterials, Photonic Crystals and Plasmonics
出版状态	已出版 - 2022
已对外发布	是
活动	12th International Conference on Metamaterials, Photonic Crystals and Plasmonics, META 2022 - Torremolinos, 西班牙期限: 19 7月 2022 → 22 7月 2022

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引用此

@article{47e77fe62f544990ad3d6b9ff787164a,

title = "Continuous-Wave mid-Infrared to Visible Frequency Upconversion with a Molecular Optomechanical Nanocavity",

abstract = "We develop a plasmonic nanoparticle-in-groove nanocavity coupled with a few hundred molecules, demonstrating optomechanical transduction of sub-microwatt continuous wave signals from the mid-infrared (32 THz) onto the visible domain at ambient conditions. The dual resonant nanocavity offers an estimated 13 orders of magnitude enhancement in upconversion efficiency per molecule. Our results establish molecular cavity optomechanics as a new paradigm for coherent frequency conversion free of phase matching constraints.",

author = "W. Chen and P. Roelli and H. Hu and S. Verlekar and Amirtharaj, \{S. P.\} and Barreda, \{A. I.\} and Kippenberg, \{T. J.\} and M. Kovylina and E. Verhagen and A. Mart{\'i}nez and C. Galland",

note = "Publisher Copyright: {\textcopyright} 2023, META Conference. All rights reserved.; 12th International Conference on Metamaterials, Photonic Crystals and Plasmonics, META 2022 ; Conference date: 19-07-2022 Through 22-07-2022",

year = "2022",

language = "英语",

pages = "703--704",

journal = "International Conference on Metamaterials, Photonic Crystals and Plasmonics",

issn = "2429-1390",

publisher = "META Conference",

}

TY - JOUR

T1 - Continuous-Wave mid-Infrared to Visible Frequency Upconversion with a Molecular Optomechanical Nanocavity

AU - Chen, W.

AU - Roelli, P.

AU - Hu, H.

AU - Verlekar, S.

AU - Amirtharaj, S. P.

AU - Barreda, A. I.

AU - Kippenberg, T. J.

AU - Kovylina, M.

AU - Verhagen, E.

AU - Martínez, A.

AU - Galland, C.

PY - 2022

Y1 - 2022

N2 - We develop a plasmonic nanoparticle-in-groove nanocavity coupled with a few hundred molecules, demonstrating optomechanical transduction of sub-microwatt continuous wave signals from the mid-infrared (32 THz) onto the visible domain at ambient conditions. The dual resonant nanocavity offers an estimated 13 orders of magnitude enhancement in upconversion efficiency per molecule. Our results establish molecular cavity optomechanics as a new paradigm for coherent frequency conversion free of phase matching constraints.

AB - We develop a plasmonic nanoparticle-in-groove nanocavity coupled with a few hundred molecules, demonstrating optomechanical transduction of sub-microwatt continuous wave signals from the mid-infrared (32 THz) onto the visible domain at ambient conditions. The dual resonant nanocavity offers an estimated 13 orders of magnitude enhancement in upconversion efficiency per molecule. Our results establish molecular cavity optomechanics as a new paradigm for coherent frequency conversion free of phase matching constraints.

UR - https://www.scopus.com/pages/publications/85179877065

M3 - 会议文章

AN - SCOPUS:85179877065

SN - 2429-1390

SP - 703

EP - 704

JO - International Conference on Metamaterials, Photonic Crystals and Plasmonics

JF - International Conference on Metamaterials, Photonic Crystals and Plasmonics

T2 - 12th International Conference on Metamaterials, Photonic Crystals and Plasmonics, META 2022

Y2 - 19 July 2022 through 22 July 2022

ER -

Continuous-Wave mid-Infrared to Visible Frequency Upconversion with a Molecular Optomechanical Nanocavity

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