TY - JOUR
T1 - Aerosol particles at a high-altitude site on the Southeast Tibetan Plateau, China
T2 - Implications for pollution transport from South Asia
AU - Zhao, Zhuzi
AU - Cao, Junji
AU - Shen, Zhenxing
AU - Xu, Baiqing
AU - Zhu, Chongshu
AU - Chen, L. W.Antony
AU - Su, Xiaoli
AU - Liu, Suixin
AU - Han, Yongming
AU - Wang, Gehui
AU - Ho, Kinfai
PY - 2013/10/16
Y1 - 2013/10/16
N2 - Bulk aerosol samples were collected from 16 July 2008 to 26 July 2009 at Lulang, a high-altitude (>3300m above sea level) site on the southeast Tibetan Plateau (TP); objectives were to determine chemical characteristics of the aerosol and identify its major sources. We report aerosol (total suspended particulate, TSP) mass levels and the concentrations of selected elements, carbonaceous species, and water-soluble inorganic ions. Significant buildup of aerosol mass and chemical species (organic carbon, element carbon, nitrate, and sulfate) occurred during the premonsoon, while lower concentrations were observed during the monsoon. Seasonal variations in aerosol and chemical species were driven by precipitation scavenging and atmospheric circulation. Two kinds of high-aerosol episodes were observed: one was enriched with dust indicators (Fe and Ca2+), and the other was enhanced with organic and elemental carbon (OC and EC), SO42-, NO3-, and Fe. The TSP loadings during the latter were 3 to 6 times those on normal days. The greatest aerosol optical depths (National Centers for Environmental Protection/National Center for Atmospheric Research reanalysis) occurred upwind, in eastern India and Bangladesh, and trajectory analysis indicates that air pollutants were transported from the southwest. Northwesterly winds brought high levels of natural emissions (Fe, Ca2+) and low levels of pollutants (SO42-, NO3-, K+, and EC); this was consistent with high aerosol optical depths over the western deserts and Gobi. Our work provides evidence that both geological and pollution aerosols from surrounding regions impact the aerosol population of the TP. Key Points One year continuous observation was carried out in southeast TP above 3300 m asl Two kinds of episodes were observed with high TSP and typical species levels Southeast TP is influenced by aerosols transported from surrounding regions
AB - Bulk aerosol samples were collected from 16 July 2008 to 26 July 2009 at Lulang, a high-altitude (>3300m above sea level) site on the southeast Tibetan Plateau (TP); objectives were to determine chemical characteristics of the aerosol and identify its major sources. We report aerosol (total suspended particulate, TSP) mass levels and the concentrations of selected elements, carbonaceous species, and water-soluble inorganic ions. Significant buildup of aerosol mass and chemical species (organic carbon, element carbon, nitrate, and sulfate) occurred during the premonsoon, while lower concentrations were observed during the monsoon. Seasonal variations in aerosol and chemical species were driven by precipitation scavenging and atmospheric circulation. Two kinds of high-aerosol episodes were observed: one was enriched with dust indicators (Fe and Ca2+), and the other was enhanced with organic and elemental carbon (OC and EC), SO42-, NO3-, and Fe. The TSP loadings during the latter were 3 to 6 times those on normal days. The greatest aerosol optical depths (National Centers for Environmental Protection/National Center for Atmospheric Research reanalysis) occurred upwind, in eastern India and Bangladesh, and trajectory analysis indicates that air pollutants were transported from the southwest. Northwesterly winds brought high levels of natural emissions (Fe, Ca2+) and low levels of pollutants (SO42-, NO3-, K+, and EC); this was consistent with high aerosol optical depths over the western deserts and Gobi. Our work provides evidence that both geological and pollution aerosols from surrounding regions impact the aerosol population of the TP. Key Points One year continuous observation was carried out in southeast TP above 3300 m asl Two kinds of episodes were observed with high TSP and typical species levels Southeast TP is influenced by aerosols transported from surrounding regions
KW - Tibetan Plateau
KW - aerosol
KW - chemical composition
KW - transport
UR - https://www.scopus.com/pages/publications/84887189989
U2 - 10.1002/jgrd.50599
DO - 10.1002/jgrd.50599
M3 - 文章
AN - SCOPUS:84887189989
SN - 2169-897X
VL - 118
SP - 11,360-11,375
JO - Journal of Geophysical Research: Atmospheres
JF - Journal of Geophysical Research: Atmospheres
IS - 19
ER -