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Ultrafast gain dynamics in N2+ lasing from highly excited vibrational states pumped by circularly polarized femtosecond laser pulses

  • Kaixuan Zhai
  • , Ziting Li
  • , Hongqiang Xie
  • , Chenrui Jing
  • , Guihua Li
  • , Bin Zeng
  • , Wei Chu
  • , Jielei Ni
  • , Jinping Yao*
  • , Ya Cheng
  • *Corresponding author for this work
  • CAS - Shanghai Institute of Optics and Fine Mechanics
  • University of Chinese Academy of Sciences
  • Tongji University

Research output: Contribution to journalArticlepeer-review

Abstract

We experimentally demonstrate N2+ lasing actions at the wavelengths of 353.3, 353.8, and 354.9 nm using a circularly polarized femtosecond laser. The three laser lines correspond to the B2Ʃu+ (v'=5, 4, 3) →X2Ʃg+ (v'=4,3,2) transitions, respectively. Particularly, we reveal the pressure-dependent gain dynamics of these lasing actions from highly excited vibrational states with a pump-Cprobe scheme. Our experimental results confirm that electron collisional excitation plays an important role in the establishment of a population inversion of N2+ lasing at these wavelengths.

Original languageEnglish
Article number050201
JournalChinese Optics Letters
Volume13
Issue number5
DOIs
StatePublished - 10 May 2015
Externally publishedYes

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