Abstract
We experimentally demonstrate third-harmonic generation (THG) by intense femtosecond laser pulse at a central wavelength of ∼800 nm superposed by its second harmonic in air. The third-harmonic signal shows a periodic modulation with a period of ∼0.67 fs when the delay between fundamental and second-harmonic wave is continuously changed. The periodic modulation of THG can be attributed to the interference of third-harmonic signals generated from a direct THG channel (3ω=ω+ω+ω) and a four-wave mixing (FWM) channel (3ω=2ω+2ω-ω). With high pump intensity, the fitting of the measured TH spectrum as a function of delay implies that the pump pulse undergoes a strong pulse splitting and self-phase modulation at the focus.
| Original language | English |
|---|---|
| Pages (from-to) | 909-912 |
| Number of pages | 4 |
| Journal | Applied Physics B: Lasers and Optics |
| Volume | 104 |
| Issue number | 4 |
| DOIs | |
| State | Published - Sep 2011 |
| Externally published | Yes |