Third-harmonic generation in relative-phase-controlled two-color laser field

H. Xu, W. Chu, Y. Liu, W. Liu, H. Xiong, Y. Fu, J. Yao, B. Zeng, J. Ni, S. L. Chin, Y. Cheng, Z. Xu

Research output: Contribution to journalArticlepeer-review

8 Scopus citations

Abstract

We experimentally demonstrate third-harmonic generation (THG) by intense femtosecond laser pulse at a central wavelength of ∼800 nm superposed by its second harmonic in air. The third-harmonic signal shows a periodic modulation with a period of ∼0.67 fs when the delay between fundamental and second-harmonic wave is continuously changed. The periodic modulation of THG can be attributed to the interference of third-harmonic signals generated from a direct THG channel (3ω=ω+ω+ω) and a four-wave mixing (FWM) channel (3ω=2ω+2ω-ω). With high pump intensity, the fitting of the measured TH spectrum as a function of delay implies that the pump pulse undergoes a strong pulse splitting and self-phase modulation at the focus.

Original languageEnglish
Pages (from-to)909-912
Number of pages4
JournalApplied Physics B: Lasers and Optics
Volume104
Issue number4
DOIs
StatePublished - Sep 2011
Externally publishedYes

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