Synthesis of Cu2MnSnS4 thin film deposited on seeded fluorine doped tin oxide substrate via a green and low-cost electrodeposition method

Jiejin Yu; Hongmei Deng; Jiahua Tao; Leilei Chen; Huiyi Cao; Lin Sun; Pingxiong Yang; Junhao Chu

doi:10.1016/j.matlet.2016.12.067

Synthesis of Cu₂MnSnS₄ thin film deposited on seeded fluorine doped tin oxide substrate via a green and low-cost electrodeposition method

Jiejin Yu
, Hongmei Deng
, Jiahua Tao
, Leilei Chen
, Huiyi Cao
, Lin Sun
, Pingxiong Yang^*
, Junhao Chu

^*Corresponding author for this work

School of Physics and Electronic Science

Research output: Contribution to journal › Article › peer-review

27 Scopus citations

Abstract

Cu₂MnSnS₄ (CMTS) thin film was the first time to deposit on the seeded fluorine doped tin oxide (FTO) substrate via sulfurization of electrodeposited Cu-Sn/Mn metal precursors. X-ray diffraction patterns and Raman measurements reveal the formation of stannite structure CMTS film with pure phase. The morphological and chemical composition studies indicate the formation of compact and homogenous CMTS thin film with Cu-poor and Mn-rich composition. The band gap of CMTS thin film is evaluated to be about 1.35 eV by the transmission spectrum. The results offer a novel research direction for preparing pure-sulfide CMTS thin films by using a simple, facile, green and low-cost electrodeposition method.

Original language	English
Pages (from-to)	186-188
Number of pages	3
Journal	Materials Letters
Volume	191
DOIs	https://doi.org/10.1016/j.matlet.2016.12.067
State	Published - 15 Mar 2017

Keywords

CuMnSnS
Electrodeposition
FTO
Semiconductors
Thin films

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10.1016/j.matlet.2016.12.067

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@article{5df7fe3bcce049278fc847cbc4c77170,

title = "Synthesis of Cu2MnSnS4 thin film deposited on seeded fluorine doped tin oxide substrate via a green and low-cost electrodeposition method",

abstract = "Cu2MnSnS4 (CMTS) thin film was the first time to deposit on the seeded fluorine doped tin oxide (FTO) substrate via sulfurization of electrodeposited Cu-Sn/Mn metal precursors. X-ray diffraction patterns and Raman measurements reveal the formation of stannite structure CMTS film with pure phase. The morphological and chemical composition studies indicate the formation of compact and homogenous CMTS thin film with Cu-poor and Mn-rich composition. The band gap of CMTS thin film is evaluated to be about 1.35 eV by the transmission spectrum. The results offer a novel research direction for preparing pure-sulfide CMTS thin films by using a simple, facile, green and low-cost electrodeposition method.",

keywords = "CuMnSnS, Electrodeposition, FTO, Semiconductors, Thin films",

author = "Jiejin Yu and Hongmei Deng and Jiahua Tao and Leilei Chen and Huiyi Cao and Lin Sun and Pingxiong Yang and Junhao Chu",

note = "Publisher Copyright: {\textcopyright} 2016 Elsevier B.V.",

year = "2017",

month = mar,

day = "15",

doi = "10.1016/j.matlet.2016.12.067",

language = "英语",

volume = "191",

pages = "186--188",

journal = "Materials Letters",

issn = "0167-577X",

publisher = "Elsevier B.V.",

}

TY - JOUR

T1 - Synthesis of Cu2MnSnS4 thin film deposited on seeded fluorine doped tin oxide substrate via a green and low-cost electrodeposition method

AU - Yu, Jiejin

AU - Deng, Hongmei

AU - Tao, Jiahua

AU - Chen, Leilei

AU - Cao, Huiyi

AU - Sun, Lin

AU - Yang, Pingxiong

AU - Chu, Junhao

PY - 2017/3/15

Y1 - 2017/3/15

N2 - Cu2MnSnS4 (CMTS) thin film was the first time to deposit on the seeded fluorine doped tin oxide (FTO) substrate via sulfurization of electrodeposited Cu-Sn/Mn metal precursors. X-ray diffraction patterns and Raman measurements reveal the formation of stannite structure CMTS film with pure phase. The morphological and chemical composition studies indicate the formation of compact and homogenous CMTS thin film with Cu-poor and Mn-rich composition. The band gap of CMTS thin film is evaluated to be about 1.35 eV by the transmission spectrum. The results offer a novel research direction for preparing pure-sulfide CMTS thin films by using a simple, facile, green and low-cost electrodeposition method.

AB - Cu2MnSnS4 (CMTS) thin film was the first time to deposit on the seeded fluorine doped tin oxide (FTO) substrate via sulfurization of electrodeposited Cu-Sn/Mn metal precursors. X-ray diffraction patterns and Raman measurements reveal the formation of stannite structure CMTS film with pure phase. The morphological and chemical composition studies indicate the formation of compact and homogenous CMTS thin film with Cu-poor and Mn-rich composition. The band gap of CMTS thin film is evaluated to be about 1.35 eV by the transmission spectrum. The results offer a novel research direction for preparing pure-sulfide CMTS thin films by using a simple, facile, green and low-cost electrodeposition method.

KW - CuMnSnS

KW - Electrodeposition

KW - FTO

KW - Semiconductors

KW - Thin films

UR - https://www.scopus.com/pages/publications/85009348027

U2 - 10.1016/j.matlet.2016.12.067

DO - 10.1016/j.matlet.2016.12.067

M3 - 文章

AN - SCOPUS:85009348027

SN - 0167-577X

VL - 191

SP - 186

EP - 188

JO - Materials Letters

JF - Materials Letters

ER -

Synthesis of Cu₂MnSnS₄ thin film deposited on seeded fluorine doped tin oxide substrate via a green and low-cost electrodeposition method

Abstract

Keywords

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