Structural reconstruction: A milestone in the hydrothermal synthesis of highly active Sn-Beta zeolites

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Abstract

A novel structural reconstruction strategy is proposed to prepare an active Sn-Beta catalyst with high Sn contents and a hydrophobic nature. Compared with post-synthesized Sn-Beta and state-of-the-art classic fluoride-mediated Sn-Beta-F, this Sn-Beta zeolite exhibits unparalleled active site-based turnover frequency for desirable products and in particular catalyst weight-based space-time-yields in various redox reactions of ketones.

Original languageEnglish
Pages (from-to)12516-12519
Number of pages4
JournalChemical Communications
Volume53
Issue number93
DOIs
StatePublished - 2017

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