Simultaneous Al2O3 doping and sulfation in hierarchically porous ZrO2 solid acids by an one-pot synthesis for enhanced recycling catalytic performances

Nan Wang; Yu Chen; Zhengqing Ye; Hangrong Chen; Jianlin Shi

doi:10.1002/cjoc.201190109

Simultaneous Al₂O₃ doping and sulfation in hierarchically porous ZrO₂ solid acids by an one-pot synthesis for enhanced recycling catalytic performances

Nan Wang^*
, Yu Chen
, Zhengqing Ye
, Hangrong Chen
, Jianlin Shi

^*Corresponding author for this work

CAS - Shanghai Institute of Ceramics

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

Alumina doping and sulfation in hierarchically porous zirconia solid acids have been achieved simultaneously via one-pot and bi-surfactant-assisted self-assembly process, using aluminum sulfate as both Al and SO₄ ^2- sources. The prepared composite solid acids showed much enhanced acidity and recycling catalytic activity for an esterification reaction compared with sulfated zirconia without alumina doping and Al-doped sulfated zirconia without hierarchically porous structure.

Original language	English
Pages (from-to)	483-488
Number of pages	6
Journal	Chinese Journal of Chemistry
Volume	29
Issue number	3
DOIs	https://doi.org/10.1002/cjoc.201190109
State	Published - Mar 2011
Externally published	Yes

Keywords

Al-promoted sulfated zirconia
Doping
Hierarchical porous structure
Material science
One-pot synthesis
Self-assembly

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10.1002/cjoc.201190109

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title = "Simultaneous Al2O3 doping and sulfation in hierarchically porous ZrO2 solid acids by an one-pot synthesis for enhanced recycling catalytic performances",

abstract = "Alumina doping and sulfation in hierarchically porous zirconia solid acids have been achieved simultaneously via one-pot and bi-surfactant-assisted self-assembly process, using aluminum sulfate as both Al and SO4 2- sources. The prepared composite solid acids showed much enhanced acidity and recycling catalytic activity for an esterification reaction compared with sulfated zirconia without alumina doping and Al-doped sulfated zirconia without hierarchically porous structure.",

keywords = "Al-promoted sulfated zirconia, Doping, Hierarchical porous structure, Material science, One-pot synthesis, Self-assembly",

author = "Nan Wang and Yu Chen and Zhengqing Ye and Hangrong Chen and Jianlin Shi",

year = "2011",

month = mar,

doi = "10.1002/cjoc.201190109",

language = "英语",

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pages = "483--488",

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T1 - Simultaneous Al2O3 doping and sulfation in hierarchically porous ZrO2 solid acids by an one-pot synthesis for enhanced recycling catalytic performances

AU - Wang, Nan

AU - Chen, Yu

AU - Ye, Zhengqing

AU - Chen, Hangrong

AU - Shi, Jianlin

PY - 2011/3

Y1 - 2011/3

N2 - Alumina doping and sulfation in hierarchically porous zirconia solid acids have been achieved simultaneously via one-pot and bi-surfactant-assisted self-assembly process, using aluminum sulfate as both Al and SO4 2- sources. The prepared composite solid acids showed much enhanced acidity and recycling catalytic activity for an esterification reaction compared with sulfated zirconia without alumina doping and Al-doped sulfated zirconia without hierarchically porous structure.

AB - Alumina doping and sulfation in hierarchically porous zirconia solid acids have been achieved simultaneously via one-pot and bi-surfactant-assisted self-assembly process, using aluminum sulfate as both Al and SO4 2- sources. The prepared composite solid acids showed much enhanced acidity and recycling catalytic activity for an esterification reaction compared with sulfated zirconia without alumina doping and Al-doped sulfated zirconia without hierarchically porous structure.

KW - Al-promoted sulfated zirconia

KW - Doping

KW - Hierarchical porous structure

KW - Material science

KW - One-pot synthesis

KW - Self-assembly

UR - https://www.scopus.com/pages/publications/79953235642

U2 - 10.1002/cjoc.201190109

DO - 10.1002/cjoc.201190109

M3 - 文章

AN - SCOPUS:79953235642

SN - 1001-604X

VL - 29

SP - 483

EP - 488

JO - Chinese Journal of Chemistry

JF - Chinese Journal of Chemistry

IS - 3

ER -

Simultaneous Al₂O₃ doping and sulfation in hierarchically porous ZrO₂ solid acids by an one-pot synthesis for enhanced recycling catalytic performances

Abstract

Keywords

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