Sediment geochemistry of Lake Daihai, north-central China: Implications for catchment weathering and climate change during the Holocene

  • Qianli Sun*
  • , Sumin Wang
  • , Jie Zhou
  • , Zhongyuan Chen
  • , Ji Shen
  • , Xiuping Xie
  • , Feng Wu
  • , Peng Chen
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

71 Scopus citations

Abstract

A 12.87-m-long sediment core was retrieved from closed-basin Lake Daihai in the monsoon-arid transition zone of north-central China. Oxides of major elements and their ratios normalized to Al in the AMS-14C-dated core were employed to evaluate chemical weathering intensity (CWI) in the lake drainage basin, which reflects hydrothermal conditions in the study area. Lower CWI periods occurred prior to 14. 5 ka BP, and during the intervals ca. 11.7-10.3, 3.5-3.2, 2.6-1.7 ka BP, and 1.2-0 ka BP, indicating relatively low temperatures and moisture availability. Greater CWI during the intervening periods ca. 14.5-11.7, 10.3-9.0, 3.2-2.6, and 1.7-1.2 ka BP, with the maximum CWI at ca. 6.7-3.5 ka BP, imply ameliorated hydrothermal conditions in the lake basin, i. e. higher temperatures and precipitation. Exceptionally low CWI, associated with high CaO/MgO ratio during ca. 9.0-6.7 ka BP, suggests higher evaporation rates in the area under warmer temperature. Overall, CWI displays in-phase variations with changes in organic matter (TOC, TN), carbonate (CaCO3) and pollen assemblages, all of which are related to variations in monsoon effective precipitation. High CWI indicates strong monsoon-induced precipitation, whereas low CWI reflects a weak precipitation regime. The optimum hydrothermal status, recorded by the strongest CWI and maximum monsoon effective precipitation during ca. 6.7-3.5 ka BP defines the Holocene climate optimum (HCO) in the Lake Daihai region. These results indicate that the HCO prevails after the early Holocene in the monsoon-arid transition zone of north-central China. Temperature and precipitation variations during most of the Holocene, inferred from the lake sediments, are due largely to insolation forcing. Dry but warm conditions ca. 9.0-6.7 ka BP, however, probably reflect the complex interactions between insolation and geography (e. g. altitude and local topography).

Original languageEnglish
Pages (from-to)75-87
Number of pages13
JournalJournal of Paleolimnology
Volume43
Issue number1
DOIs
StatePublished - 2010
Externally publishedYes

Keywords

  • Chemical weathering
  • Effective precipitation
  • Hydrothermal status
  • Lake Daihai
  • Major elements

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