Optimal spectral phase control of femtosecond laser-induced up-conversion luminescence in Sm3+:NaYF4 glass

Jian Ping Li; Lian Zhong Deng; Ye Zheng; Peng Peng Ding; Tian Qing Jia; Zhen Rong Sun; Jian Rong Qiu; Shi An Zhang

doi:10.1007/s11467-019-0947-7

Optimal spectral phase control of femtosecond laser-induced up-conversion luminescence in Sm³⁺:NaYF₄ glass

Jian Ping Li
, Lian Zhong Deng^*
, Ye Zheng
, Peng Peng Ding
, Tian Qing Jia
, Zhen Rong Sun
, Jian Rong Qiu
, Shi An Zhang

^*Corresponding author for this work

Institute for Advanced Study in Precision Spectroscopy

Research output: Contribution to journal › Article › peer-review

10 Scopus citations

Abstract

The spectral phase of the femtosecond laser field is an important parameter that affects the upconversion (UC) luminescence efficiency of dopant lanthanide ions. In this work, we report an experimental study on controlling the UC luminescence efficiency in Sm³⁺:NaYF₄ glass by 800-nm femtosecond laser pulse shaping using spectral phase modulation. The optimal phase control strategy efficiently enhances or suppresses the UC luminescence intensity. Based on the laser-power dependence of the UC luminescence intensity and its comparison with the luminescence spectrum under direct 266-nm femtosecond laser irradiation, we propose herein an excitation model combining non-resonant two-photon absorption with resonance-mediated three-photon absorption to explain the experimental observations.

Original language	English
Article number	22603
Journal	Frontiers of Physics
Volume	15
Issue number	2
DOIs	https://doi.org/10.1007/s11467-019-0947-7
State	Published - 1 Apr 2020

Keywords

femtosecond laser
quantum control
rare earth ions
spectral phase
up-conversion luminescence

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10.1007/s11467-019-0947-7

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title = "Optimal spectral phase control of femtosecond laser-induced up-conversion luminescence in Sm3+:NaYF4 glass",

abstract = "The spectral phase of the femtosecond laser field is an important parameter that affects the upconversion (UC) luminescence efficiency of dopant lanthanide ions. In this work, we report an experimental study on controlling the UC luminescence efficiency in Sm3+:NaYF4 glass by 800-nm femtosecond laser pulse shaping using spectral phase modulation. The optimal phase control strategy efficiently enhances or suppresses the UC luminescence intensity. Based on the laser-power dependence of the UC luminescence intensity and its comparison with the luminescence spectrum under direct 266-nm femtosecond laser irradiation, we propose herein an excitation model combining non-resonant two-photon absorption with resonance-mediated three-photon absorption to explain the experimental observations.",

keywords = "femtosecond laser, quantum control, rare earth ions, spectral phase, up-conversion luminescence",

author = "Li, \{Jian Ping\} and Deng, \{Lian Zhong\} and Ye Zheng and Ding, \{Peng Peng\} and Jia, \{Tian Qing\} and Sun, \{Zhen Rong\} and Qiu, \{Jian Rong\} and Zhang, \{Shi An\}",

note = "Publisher Copyright: {\textcopyright} 2020, Higher Education Press and Springer-Verlag GmbH Germany, part of Springer Nature.",

year = "2020",

month = apr,

day = "1",

doi = "10.1007/s11467-019-0947-7",

language = "英语",

volume = "15",

journal = "Frontiers of Physics",

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T1 - Optimal spectral phase control of femtosecond laser-induced up-conversion luminescence in Sm3+:NaYF4 glass

AU - Li, Jian Ping

AU - Deng, Lian Zhong

AU - Zheng, Ye

AU - Ding, Peng Peng

AU - Jia, Tian Qing

AU - Sun, Zhen Rong

AU - Qiu, Jian Rong

AU - Zhang, Shi An

PY - 2020/4/1

Y1 - 2020/4/1

N2 - The spectral phase of the femtosecond laser field is an important parameter that affects the upconversion (UC) luminescence efficiency of dopant lanthanide ions. In this work, we report an experimental study on controlling the UC luminescence efficiency in Sm3+:NaYF4 glass by 800-nm femtosecond laser pulse shaping using spectral phase modulation. The optimal phase control strategy efficiently enhances or suppresses the UC luminescence intensity. Based on the laser-power dependence of the UC luminescence intensity and its comparison with the luminescence spectrum under direct 266-nm femtosecond laser irradiation, we propose herein an excitation model combining non-resonant two-photon absorption with resonance-mediated three-photon absorption to explain the experimental observations.

AB - The spectral phase of the femtosecond laser field is an important parameter that affects the upconversion (UC) luminescence efficiency of dopant lanthanide ions. In this work, we report an experimental study on controlling the UC luminescence efficiency in Sm3+:NaYF4 glass by 800-nm femtosecond laser pulse shaping using spectral phase modulation. The optimal phase control strategy efficiently enhances or suppresses the UC luminescence intensity. Based on the laser-power dependence of the UC luminescence intensity and its comparison with the luminescence spectrum under direct 266-nm femtosecond laser irradiation, we propose herein an excitation model combining non-resonant two-photon absorption with resonance-mediated three-photon absorption to explain the experimental observations.

KW - femtosecond laser

KW - quantum control

KW - rare earth ions

KW - spectral phase

KW - up-conversion luminescence

UR - https://www.scopus.com/pages/publications/85077901442

U2 - 10.1007/s11467-019-0947-7

DO - 10.1007/s11467-019-0947-7

M3 - 文章

AN - SCOPUS:85077901442

SN - 2095-0462

VL - 15

JO - Frontiers of Physics

JF - Frontiers of Physics

IS - 2

M1 - 22603

ER -

Optimal spectral phase control of femtosecond laser-induced up-conversion luminescence in Sm³⁺:NaYF₄ glass

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Keywords

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