Observation of the Interlayer Exciton Gases in WSe2-p:WSe2Heterostructures

  • Zheng Sun*
  • , Jonathan Beaumariage
  • , Qingrui Cao
  • , Kenji Watanabe
  • , Takashi Taniguchi
  • , Benjamin Matthew Hunt
  • , David Snoke
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

6 Scopus citations

Abstract

Interlayer excitons (IXs) possess a much longer lifetime than intralayer excitons due to the spatial separation of the electrons and holes, and hence they have been pursued to create exciton condensates for decades. The recent emergence of 2D materials, such as transition-metal dichalcogenides (TMDs), and of their van der Waals heterostructures, in which two different 2D materials are layered together, has created new opportunities to study IXs. Here we present the observation of IX gases within two stacked structures consisting of hBN/WSe2/hBN/p:WSe2/hBN. The IX energies of the two different structures differed by 82 meV due to the different thicknesses of the hexagonal boron nitride spacer layer between the TMD layers. We demonstrate that the lifetime of the IXs is shortened when the temperature and the pump power increase. We attribute this nonlinear behavior to an Auger process.

Original languageEnglish
Pages (from-to)1622-1627
Number of pages6
JournalACS Photonics
Volume7
Issue number7
DOIs
StatePublished - 15 Jul 2020
Externally publishedYes

Keywords

  • Auger process
  • homobilayers
  • interlayer excitons
  • lifetime
  • thermal distribution

Fingerprint

Dive into the research topics of 'Observation of the Interlayer Exciton Gases in WSe2-p:WSe2Heterostructures'. Together they form a unique fingerprint.

Cite this