Mid-infrared photon counting and resolving via efficient frequency upconversion

Optical detectors with single-photon sensitivity and large dynamic range would facilitate a variety of applications. Specifically, the capability of extending operation wavelengths into the mid-infrared region is highly attractive. Here we implement a mid-infrared frequency upconversion detector for counting and resolving photons at 3 μm. Thanks to the spectrotemporal engineering of the involved optical fields, the mid-infrared photons could be spectrally translated into the visible band with a conversion efficiency of 80%. In combination with a silicon avalanche photodiode, we obtained unprecedented performance with a high overall detection efficiency of 37% and a low noise equivalent power of 1.8 × 10−¹⁷ W∕Hz¹∕². Furthermore, photon-number-resolving detection at mid-infrared wavelengths was demonstrated, for the first time to our knowledge, with a multipixel photon counter. The implemented upconversion detector exhibited a maximal resolving photon number up to 9 with a noise probability per pulse of 0.14% at the peak detection efficiency. The achieved photon counting and resolving performance might open up new possibilities in trace molecule spectroscopy, sensitive biochemical sensing, and free-space communications, among others.