Iso-butanol dehydration by pervaporation using zeolite LTA membranes prepared on 3-aminopropyltriethoxysilane-modified alumina tubes

Bingxin Huang; Qian Liu; Jürgen Caro; Aisheng Huang

doi:10.1016/j.memsci.2013.12.075

Iso-butanol dehydration by pervaporation using zeolite LTA membranes prepared on 3-aminopropyltriethoxysilane-modified alumina tubes

Bingxin Huang
, Qian Liu
, Jürgen Caro
, Aisheng Huang^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

58 Scopus citations

Abstract

Dense and phase-pure zeolite LTA membranes were hydrothermally synthesized on 3-aminopropyltriethoxysilane (APTES)-modified macroporous Al₂O₃ tubes without seeding. Pervaporation experiments were conducted for the separation of liquid water/iso-butanol and water/ethanol mixtures to evaluate the separation performances of the zeolite LTA membranes. A water flux of 4.5kg/m²h is obtained at 100°C for the separation of a 95.0wt% iso-butanol/5.0wt% water mixture, and the separation factors of water/iso-butanol are found to be about 3000 for all temperatures and concentrations studied.

Original language	English
Pages (from-to)	200-206
Number of pages	7
Journal	Journal of Membrane Science
Volume	455
DOIs	https://doi.org/10.1016/j.memsci.2013.12.075
State	Published - 1 Apr 2014
Externally published	Yes

Keywords

Hydrothermal synthesis
Pervaporation
Water/iso-butanol dehydration
Zeolite LTA membrane

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10.1016/j.memsci.2013.12.075

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title = "Iso-butanol dehydration by pervaporation using zeolite LTA membranes prepared on 3-aminopropyltriethoxysilane-modified alumina tubes",

abstract = "Dense and phase-pure zeolite LTA membranes were hydrothermally synthesized on 3-aminopropyltriethoxysilane (APTES)-modified macroporous Al2O3 tubes without seeding. Pervaporation experiments were conducted for the separation of liquid water/iso-butanol and water/ethanol mixtures to evaluate the separation performances of the zeolite LTA membranes. A water flux of 4.5kg/m2h is obtained at 100°C for the separation of a 95.0wt\% iso-butanol/5.0wt\% water mixture, and the separation factors of water/iso-butanol are found to be about 3000 for all temperatures and concentrations studied.",

keywords = "Hydrothermal synthesis, Pervaporation, Water/iso-butanol dehydration, Zeolite LTA membrane",

author = "Bingxin Huang and Qian Liu and J{\"u}rgen Caro and Aisheng Huang",

year = "2014",

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doi = "10.1016/j.memsci.2013.12.075",

language = "英语",

volume = "455",

pages = "200--206",

journal = "Journal of Membrane Science",

issn = "0376-7388",

publisher = "Elsevier B.V.",

}

TY - JOUR

T1 - Iso-butanol dehydration by pervaporation using zeolite LTA membranes prepared on 3-aminopropyltriethoxysilane-modified alumina tubes

AU - Huang, Bingxin

AU - Liu, Qian

AU - Caro, Jürgen

AU - Huang, Aisheng

PY - 2014/4/1

Y1 - 2014/4/1

N2 - Dense and phase-pure zeolite LTA membranes were hydrothermally synthesized on 3-aminopropyltriethoxysilane (APTES)-modified macroporous Al2O3 tubes without seeding. Pervaporation experiments were conducted for the separation of liquid water/iso-butanol and water/ethanol mixtures to evaluate the separation performances of the zeolite LTA membranes. A water flux of 4.5kg/m2h is obtained at 100°C for the separation of a 95.0wt% iso-butanol/5.0wt% water mixture, and the separation factors of water/iso-butanol are found to be about 3000 for all temperatures and concentrations studied.

AB - Dense and phase-pure zeolite LTA membranes were hydrothermally synthesized on 3-aminopropyltriethoxysilane (APTES)-modified macroporous Al2O3 tubes without seeding. Pervaporation experiments were conducted for the separation of liquid water/iso-butanol and water/ethanol mixtures to evaluate the separation performances of the zeolite LTA membranes. A water flux of 4.5kg/m2h is obtained at 100°C for the separation of a 95.0wt% iso-butanol/5.0wt% water mixture, and the separation factors of water/iso-butanol are found to be about 3000 for all temperatures and concentrations studied.

KW - Hydrothermal synthesis

KW - Pervaporation

KW - Water/iso-butanol dehydration

KW - Zeolite LTA membrane

UR - https://www.scopus.com/pages/publications/84892973076

U2 - 10.1016/j.memsci.2013.12.075

DO - 10.1016/j.memsci.2013.12.075

M3 - 文章

AN - SCOPUS:84892973076

SN - 0376-7388

VL - 455

SP - 200

EP - 206

JO - Journal of Membrane Science

JF - Journal of Membrane Science

ER -

Iso-butanol dehydration by pervaporation using zeolite LTA membranes prepared on 3-aminopropyltriethoxysilane-modified alumina tubes

Abstract

Keywords

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