Abstract
We report on experimental realization of impulsive rotational Raman scattering from neutral nitrogen molecules in a femtosecond laser filament using an intense self-induced white-light seeding "air laser" generated during the filamentation of an 800 nm Ti:sapphire laser in nitrogen gas. The impulsive rotational Raman fingerprint signals are observed with a maximum conversion efficiency of ∼0.8%. Our observation provides a promising way of remote identification and location of chemical species in the atmosphere by a rotational Raman scattering of molecules.
| Original language | English |
|---|---|
| Pages (from-to) | 2250-2253 |
| Number of pages | 4 |
| Journal | Optics Letters |
| Volume | 39 |
| Issue number | 8 |
| DOIs | |
| State | Published - 15 Apr 2014 |
| Externally published | Yes |