Impulsive rotational Raman scattering of N2 by a remote "air laser" in femtosecond laser filament

Jielei Ni, Wei Chu, Haisu Zhang, Bin Zeng, Jinping Yao, Lingling Qiao, Guihua Li, Chenrui Jing, Hongqiang Xie, Huailiang Xu, Ya Cheng, Zhizhan Xu

Research output: Contribution to journalArticlepeer-review

40 Scopus citations

Abstract

We report on experimental realization of impulsive rotational Raman scattering from neutral nitrogen molecules in a femtosecond laser filament using an intense self-induced white-light seeding "air laser" generated during the filamentation of an 800 nm Ti:sapphire laser in nitrogen gas. The impulsive rotational Raman fingerprint signals are observed with a maximum conversion efficiency of ∼0.8%. Our observation provides a promising way of remote identification and location of chemical species in the atmosphere by a rotational Raman scattering of molecules.

Original languageEnglish
Pages (from-to)2250-2253
Number of pages4
JournalOptics Letters
Volume39
Issue number8
DOIs
StatePublished - 15 Apr 2014
Externally publishedYes

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