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Impact of sulfur doping on broadband terahertz emission in gallium selenide single crystals via optical rectification

  • Gaofang Li
  • , Renjie Huang
  • , Jingguo Huang
  • , Wenjie Zhang
  • , Haoyang Cui
  • , Nenghong Xia
  • , Zhiming Huang*
  • , Junhao Chu
  • , Guohong Ma*
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

Abstract

The impact of sulfur doping on broadband terahertz emission in GaSe single crystals was investigated by optical rectification with oo-o phase matching. The maximum peak value of THz radiation generated from S-doped 2.5 mass% GaSe is 28.3% larger than that of intrinsic GaSe with pump fluence of 637 mW cm-2 and azimuthal angle of 0o. The saturation of THz emission in S-doped 2.5 mass% GaSe is increased compared with that of intrinsic and S-doped 7 mass% GaSe. The results demonstrate that GaSe with appropriate S-doping concentration can effectively improve the broadband THz radiation and saturation.

Original languageEnglish
Article number072004
JournalApplied Physics Express
Volume14
Issue number7
DOIs
StatePublished - Jul 2021
Externally publishedYes

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