Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

H. Sann; T. Havermeier; C. Müller; H. K. Kim; F. Trinter; M. Waitz; J. Voigtsberger; F. Sturm; T. Bauer; R. Wallauer; D. Schneider; M. Weller; C. Goihl; J. Tross; K. Cole; J. Wu; M. S. Schöffler; H. Schmidt-Böcking; T. Jahnke; M. Simon; R. Dörner

doi:10.1103/PhysRevLett.117.243002

Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

H. Sann
, T. Havermeier
, C. Müller
, H. K. Kim
, F. Trinter
, M. Waitz
, J. Voigtsberger
, F. Sturm
, T. Bauer
, R. Wallauer
, D. Schneider
, M. Weller
, C. Goihl
, J. Tross
, K. Cole
, J. Wu
, M. S. Schöffler
, H. Schmidt-Böcking
, T. Jahnke
, M. Simon

R. Dörner

Goethe University Frankfurt
University of Marburg
Sorbonne Université

Research output: Contribution to journal › Article › peer-review

30 Scopus citations

Abstract

We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.

Original language	English
Article number	243002
Journal	Physical Review Letters
Volume	117
Issue number	24
DOIs	https://doi.org/10.1103/PhysRevLett.117.243002
State	Published - 6 Dec 2016
Externally published	Yes

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Sann, H., Havermeier, T., Müller, C., Kim, H. K., Trinter, F., Waitz, M., Voigtsberger, J., Sturm, F., Bauer, T., Wallauer, R., Schneider, D., Weller, M., Goihl, C., Tross, J., Cole, K., Wu, J., Schöffler, M. S., Schmidt-Böcking, H., Jahnke, T., ... Dörner, R. (2016). Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation. Physical Review Letters, 117(24), Article 243002. https://doi.org/10.1103/PhysRevLett.117.243002

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title = "Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation",

abstract = "We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.",

author = "H. Sann and T. Havermeier and C. M{\"u}ller and Kim, \{H. K.\} and F. Trinter and M. Waitz and J. Voigtsberger and F. Sturm and T. Bauer and R. Wallauer and D. Schneider and M. Weller and C. Goihl and J. Tross and K. Cole and J. Wu and Sch{\"o}ffler, \{M. S.\} and H. Schmidt-B{\"o}cking and T. Jahnke and M. Simon and R. D{\"o}rner",

note = "Publisher Copyright: {\textcopyright} 2016 American Physical Society.",

year = "2016",

month = dec,

day = "6",

doi = "10.1103/PhysRevLett.117.243002",

language = "英语",

volume = "117",

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Sann, H, Havermeier, T, Müller, C, Kim, HK, Trinter, F, Waitz, M, Voigtsberger, J, Sturm, F, Bauer, T, Wallauer, R, Schneider, D, Weller, M, Goihl, C, Tross, J, Cole, K, Wu, J, Schöffler, MS, Schmidt-Böcking, H, Jahnke, T, Simon, M & Dörner, R 2016, 'Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation', Physical Review Letters, vol. 117, no. 24, 243002. https://doi.org/10.1103/PhysRevLett.117.243002

TY - JOUR

T1 - Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

AU - Sann, H.

AU - Havermeier, T.

AU - Müller, C.

AU - Kim, H. K.

AU - Trinter, F.

AU - Waitz, M.

AU - Voigtsberger, J.

AU - Sturm, F.

AU - Bauer, T.

AU - Wallauer, R.

AU - Schneider, D.

AU - Weller, M.

AU - Goihl, C.

AU - Tross, J.

AU - Cole, K.

AU - Wu, J.

AU - Schöffler, M. S.

AU - Schmidt-Böcking, H.

AU - Jahnke, T.

AU - Simon, M.

AU - Dörner, R.

PY - 2016/12/6

Y1 - 2016/12/6

N2 - We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.

AB - We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular σ orbital to that of an atomic p state as the system evolves from a molecule into two separated atoms.

UR - https://www.scopus.com/pages/publications/85003443820

U2 - 10.1103/PhysRevLett.117.243002

DO - 10.1103/PhysRevLett.117.243002

M3 - 文章

AN - SCOPUS:85003443820

SN - 0031-9007

VL - 117

JO - Physical Review Letters

JF - Physical Review Letters

IS - 24

M1 - 243002

ER -

Imaging the Temporal Evolution of Molecular Orbitals during Ultrafast Dissociation

Abstract

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