From CuFeS2 to Ba6Cu2FeGe4S16: Rational band gap engineering achieves large second-harmonic-generation together with high laser damage threshold

Wangzhu Cao; Dajiang Mei; Yi Yang; Yuanwang Wu; Lingyun Zhang; Yuandong Wu; Xiao He; Zheshuai Lin; Fuqiang Huang

doi:10.1039/c9cc07288h

From CuFeS₂ to Ba₆Cu₂FeGe₄S₁₆: Rational band gap engineering achieves large second-harmonic-generation together with high laser damage threshold

Wangzhu Cao, Dajiang Mei, Yi Yang, Yuanwang Wu, Lingyun Zhang, Yuandong Wu, Xiao He, Zheshuai Lin, Fuqiang Huang

School of Chemistry and Molecular Engineering

Research output: Contribution to journal › Article › peer-review

24 Scopus citations

Abstract

A new germanium-based sulfide, Ba₆Cu₂FeGe₄S₁₆, achieves a band-gap broadening of more than 1 eV relative to CuFeS₂. Remarkably, Ba₆Cu₂FeGe₄S₁₆ exhibits excellent comprehensive NLO performance (SHG, 1.5 × AgGaSe₂; LDT, 2 × AgGaSe₂), satisfying the essential requirements of mid-IR NLO candidates.

Original language	English
Pages (from-to)	14510-14513
Number of pages	4
Journal	Chemical Communications
Volume	55
Issue number	96
DOIs	https://doi.org/10.1039/c9cc07288h
State	Published - 2019

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title = "From CuFeS2 to Ba6Cu2FeGe4S16: Rational band gap engineering achieves large second-harmonic-generation together with high laser damage threshold",

abstract = "A new germanium-based sulfide, Ba6Cu2FeGe4S16, achieves a band-gap broadening of more than 1 eV relative to CuFeS2. Remarkably, Ba6Cu2FeGe4S16 exhibits excellent comprehensive NLO performance (SHG, 1.5 × AgGaSe2; LDT, 2 × AgGaSe2), satisfying the essential requirements of mid-IR NLO candidates.",

author = "Wangzhu Cao and Dajiang Mei and Yi Yang and Yuanwang Wu and Lingyun Zhang and Yuandong Wu and Xiao He and Zheshuai Lin and Fuqiang Huang",

note = "Publisher Copyright: {\textcopyright} 2019 The Royal Society of Chemistry.",

year = "2019",

doi = "10.1039/c9cc07288h",

language = "英语",

volume = "55",

pages = "14510--14513",

journal = "Chemical Communications",

issn = "1359-7345",

publisher = "Royal Society of Chemistry",

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TY - JOUR

T1 - From CuFeS2 to Ba6Cu2FeGe4S16

T2 - Rational band gap engineering achieves large second-harmonic-generation together with high laser damage threshold

AU - Cao, Wangzhu

AU - Mei, Dajiang

AU - Yang, Yi

AU - Wu, Yuanwang

AU - Zhang, Lingyun

AU - Wu, Yuandong

AU - He, Xiao

AU - Lin, Zheshuai

AU - Huang, Fuqiang

PY - 2019

Y1 - 2019

N2 - A new germanium-based sulfide, Ba6Cu2FeGe4S16, achieves a band-gap broadening of more than 1 eV relative to CuFeS2. Remarkably, Ba6Cu2FeGe4S16 exhibits excellent comprehensive NLO performance (SHG, 1.5 × AgGaSe2; LDT, 2 × AgGaSe2), satisfying the essential requirements of mid-IR NLO candidates.

AB - A new germanium-based sulfide, Ba6Cu2FeGe4S16, achieves a band-gap broadening of more than 1 eV relative to CuFeS2. Remarkably, Ba6Cu2FeGe4S16 exhibits excellent comprehensive NLO performance (SHG, 1.5 × AgGaSe2; LDT, 2 × AgGaSe2), satisfying the essential requirements of mid-IR NLO candidates.

UR - https://www.scopus.com/pages/publications/85075814034

U2 - 10.1039/c9cc07288h

DO - 10.1039/c9cc07288h

M3 - 文章

C2 - 31735948

AN - SCOPUS:85075814034

SN - 1359-7345

VL - 55

SP - 14510

EP - 14513

JO - Chemical Communications

JF - Chemical Communications

IS - 96

ER -

From CuFeS₂ to Ba₆Cu₂FeGe₄S₁₆: Rational band gap engineering achieves large second-harmonic-generation together with high laser damage threshold

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