Abstract
We theoretically study the field-free molecular orientation by a multicolor laser field with a superposition of the fundamental wave and its harmonics. It is shown that the molecular orientation will be up to a maximum value pumped by the four-color laser field at the same laser intensity, and the molecular orientation direction and its degree can be controlled by varying the carrier-envelope phase of the four-color laser field. It is also indicated that the molecular orientation induced by a four-color laser field can be tremendously enhanced by applying another in-phase or out-phase four-color laser field at the beginning of the rotational wave-packet rephasing or the end of the rotational wave-packet dephasing.
| Original language | English |
|---|---|
| Article number | 023416 |
| Journal | Physical Review A - Atomic, Molecular, and Optical Physics |
| Volume | 83 |
| Issue number | 2 |
| DOIs | |
| State | Published - 22 Feb 2011 |
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