Field-free molecular orientation by a multicolor laser field

Shian Zhang, Junhui Shi, Hui Zhang, Tianqing Jia, Zugeng Wang, Zhenrong Sun

Research output: Contribution to journalArticlepeer-review

43 Scopus citations

Abstract

We theoretically study the field-free molecular orientation by a multicolor laser field with a superposition of the fundamental wave and its harmonics. It is shown that the molecular orientation will be up to a maximum value pumped by the four-color laser field at the same laser intensity, and the molecular orientation direction and its degree can be controlled by varying the carrier-envelope phase of the four-color laser field. It is also indicated that the molecular orientation induced by a four-color laser field can be tremendously enhanced by applying another in-phase or out-phase four-color laser field at the beginning of the rotational wave-packet rephasing or the end of the rotational wave-packet dephasing.

Original languageEnglish
Article number023416
JournalPhysical Review A - Atomic, Molecular, and Optical Physics
Volume83
Issue number2
DOIs
StatePublished - 22 Feb 2011

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