Double-layer heterostructure of graphene/carbon nanotube films for highly efficient broadband photodetector

Graphene-semiconducting single-wall carbon nanotubes' (graphene-s-SWCNTs) thin-film photodetector based on a double-layer stacked heterostructure was fabricated. The carbon-based heterostructure exhibits excellent long-range van der Waals interactions. The as-fabricated device was demonstrated with an ultra-broadband photodetection characteristic with a high responsivity of 78 A/W at a visible wavelength and a fast response time of 80 μs. Moreover, the high photoconductive gain based on the photogating effect for the graphene-s-SWCNTs device was realized. In addition, the temperature-dependent photoresponse performance was also demonstrated. Benefiting from the high photoconductive gain, ultra-fast response time, and high stable quality of carbon materials, our devices exhibit great potential applications for high sensitivity detection to weak target signals in extreme environments.