Deceleration of heavy atoms with a continuous stimulated force

Heavy atoms play a critical role in scientific research and applications by providing a better understanding of fundamental physical phenomena. The use of a slowed atomic beam to extend the interaction time is expected to enhance measurement sensitivity, resolution, and precision. Here, we theoretically demonstrate a rapid and short-distance deceleration of heavy atoms by using a continuous stimulated force with optical phase compensation and frequency chirping. The scheme effectively overcomes the spatial inhomogeneity of the stimulated force on atoms during deceleration. Our approach employs the numerical solutions of the optical Bloch equations for two-level atoms driven by time-dependent fields, and simulates atom trajectories using a three-dimensional Monte Carlo method. Concerning a buffer-gas-cooled radium atom beam with an initial velocity of 130 m/s, from our simulations it can be decelerated to 5 m/s within 5 cm distance using 40 mW laser power, achieving a deceleration force approximately 35 times stronger than the radiation force and covering an effective velocity range over eight times that of the radiation force. In addition, the deceleration of other heavy atoms, such as francium and thallium, also are applicable. This approach offers an efficient tool for rapidly slowing and cooling complex atoms and molecules, facilitating future precision measurements.