Abstract
We experimentally demonstrate the Coulomb explosion process of CS2 molecule under a near-infrared (800 nm) intense femtosecond laser field by a DC-sliced ion imaging technique. We obtain the DC-sliced images of these fragment ions S+, S2+, CS+, and CS2+ by breaking one C-S bond, and assign their Coulomb explosion channels by considering their kinetic energy release and angular distribution. We also numerically simulate the dissociation dynamics of parent ions CS2 k+ (k =2-4) by a Coulomb potential approximation, and obtain the time evolution of Coulomb energy and kinetic energy release, which indicates that the dissociation time of parent ions CS2 k+ decreases with the increase of the charge number k. These experimental and theoretical results can serve as a useful benchmark for those researchers who work in the related area.
| Original language | English |
|---|---|
| Article number | 053301 |
| Journal | Chinese Physics B |
| Volume | 25 |
| Issue number | 5 |
| DOIs | |
| State | Published - May 2016 |
Keywords
- Coulomb explosion
- femtosecond laser field
- molecular photodissociation