Abstract
The present paper describes a new method for manufacturing large scale, stable, transportable, and designable nanostructured porous TiO2 tapes on various substrates for use in photoelectrochemical cells. The method involves predeposition of TiO2 strips on the fluorine doped tin oxide (FTO) glass by screen-printing method, peeling off TiO2 strips from the substrate by a novel laser-assisted lift-off technique, sintering the formed TiO2 tapes at 500 C for 15 min, and compressing the sintered TiO2 tapes on different conductive substrates with a low pressure rolling press to form mechanically stable, electrically conducting, porous nanostructured TiO2 electrodes at room temperature. Photoelectrochemical characteristics of the resulted electrodes are presented. Dye-sensitized solar cells (DSSCs) with the as-fabricated TiO2 photoanodes on PET-ITO and FTO glass achieved a conversion efficiency of 4.2% and 6.2%, respectively. The potential use of this new manufacturing method in future DSSC applications is discussed.
| Original language | English |
|---|---|
| Pages (from-to) | 13000-13005 |
| Number of pages | 6 |
| Journal | ACS Applied Materials and Interfaces |
| Volume | 5 |
| Issue number | 24 |
| DOIs | |
| State | Published - 26 Dec 2013 |
| Externally published | Yes |
Keywords
- Dye-sensitized solar cell
- Laser-assisted lift-off
- Layer transfer
- Low temperature
- Rolling press
- TiO tape
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